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Abstract Within Earth's critical zone, weathering processes influence landscape evolution and hillslope hydrology by creating porosity in bedrock, transforming it into saprolite and eventually soil. In situ weathering processes drive much of this transformation while preserving the rock fabric of the parent material. Inherited rock fabric in regolith makes the critical zone anisotropic, affecting its mechanical and hydrological properties. Therefore, quantifying and studying anisotropy is an important part of characterising the critical zone, yet doing so remains challenging. Seismic methods can be used to detect rock fabric and infer mechanical and hydrologic conductivity anisotropy across landscapes. We present a novel way of measuring seismic anisotropy in the critical zone using Rayleigh and Love surface waves. This method leverages multi‐component surface seismic data to create a high‐resolution model of seismic anisotropy, which we compare with a nuclear magnetic resonance log measured in a nearby borehole. The two geophysical data sets show that seismic anisotropy and porosity develop at similar depths in weathered bedrock and both reach their maximum values in saprolite, implying that in situ weathering enhances anisotropy while concurrently generating porosity in the critical zone. We bolster our findings with in situ measurements of seismic and hydrologic conductivity anisotropy made in a 3 m deep soil excavation. Our study offers a fresh perspective on the importance of rock fabric in the development and function of the critical zone and sheds new insights into how weathering processes operate.